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Relationships between the efficiency of cyclohexane oxidation and the electrochemical parameters of the reaction solution

Relationships between the efficiency of cyclohexane oxidation and the electrochemical parameters of the reaction solution,10.1016/j.molcata.2011.07.00

Relationships between the efficiency of cyclohexane oxidation and the electrochemical parameters of the reaction solution  
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Vanadyl(IV)-acetylacetonate-catalyzed oxidation of cyclohexane with H2O2, at 40°C under air atmosphere, has been studied in the presence of small quantities of oxalic acid. The process efficiency is increased by this additive and depends on the nature of the solvent (MeCN≥MeOH>Me2CO≥2-PrOH>EtOH). The relationships between the results (conversion, yield) and the electrochemical characteristics of the reaction solution (relative permittivity, redox-potential) are highlighted and discussed.
Journal: Journal of Molecular Catalysis A-chemical - J MOL CATAL A-CHEM , vol. 347, no. 1, pp. 15-21, 2011
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